Vertical Distribution of Radioactive Particles in Ottawa River Sediment Near the Chalk River Laboratories

Abstract

Previously, we described an area of above-background levels of radioactivity in the bed of the Ottawa River near the Chalk River Laboratories. The area was about 200 m wide by 400 m long and in water 8 to 30 m deep. The source of the radioactivity was associated with the location of cooling-water discharge. Particles of radioactive material were later recovered from the upper 10-15 cm of sediment and were determined to be sand-sized grains of nuclear fuel and corrosion products.

This report provides an examination of the vertical distribution of radioactive particles in the riverbed. Twenty-three dredge samples (representing 1.2 m² of riverbed) were collected near the Process Outfall. Each dredge sample was dissected in horizontal intervals 1-cm-thick. Each interval provided a 524 cm³ sample of sediment that was carefully examined for particulate radioactivity. Approximately 80% of the radioactivity appeared to be associated with discrete particles. Although the natural sediment in the general area is cohesive, silty clay and contains less than 10% sand, the sediment near the Outfall was found to be rich in natural sand, presumably from sources such as winter sanding of roads at the laboratories. The radioactive particles were almost entirely contained in the top-most 10 cm of the river bed. The majority of the particles were found several centimetres beneath the sediment surface and the numbers of particles and the radioactivity of the particles peaked 3 to 7 cm below the sediment surface. Based on the sediment profile, there appeared to have been a marked decrease in the deposition of particulate radioactivity in recent decades. The vertical distribution of radioactive particles indicated that sedimentation is resulting in burial and that the deposition of most of the particulate radioactivity coincided with the operation of Chalk River’s NRX reactor from 1947 to 1992.